Chloromethyl-triazole: a new motif for site-selective pseudo-acylation of proteins

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Chloromethyl-triazole: a new motif for site-selective pseudo-acylation of proteins† †Electronic supplementary information (ESI) available: Synthesis and characterisation of compounds 3b, 4b, and peptides Pep1–3. Peptide and protein alkylation procedures. See DOI: 10.1039/c6cc06801d. Primary data files can be found at http://dx.doi.org/10.7488/ds/1484 Click here for additional data file.

Rapid, site-selective modification of cysteine residues with chloromethyl-triazole derivatives generates pseudo-acyl sLys motifs, mimicking important post-translational modifications. Near-native biotinylation of peptide and protein substrates is shown to be site-selective and modified histone H4 retains functional activity.

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ژورنال

عنوان ژورنال: Chemical Communications

سال: 2016

ISSN: 1359-7345,1364-548X

DOI: 10.1039/c6cc06801d